So you are using vintage Altec Voice of the theater components.
In a home it will be had to get far enough away from them. They were designed for large spaces..
The horns are pretty fierce by modern standards.
The passive crossovers are pretty poor. In the best cinemas they were always biamped.
Shure made an electronic crossover that suited them well. It is the Shure SR 106.
You can select crossover points of 500 Hz, 800 Hz or 2600 HZ. for the voice of the theater range the 800 Hz setting works best. The low pass is first order and the high pass second order.
You will need one for each channel, and two power amps for each speaker. If the amps do not have level controls you will need to add them, between at least the crossover high pass and the HF power amp.
This set up totally transforms the Voice of the Theater systems.
These systems were built for high sensitivity as the amps were tube and not high powered by modern standards. This means that the bass turnover point was around 60 Hz.
So I would leave the speakers set to large and add the sub starting around 80 Hz. You can also try 60 Hz and see which sounds the best.