I have Klipsch RF-3's (37Hz-20kHz(+-)3dB) and I run them full range because I seldom use my subwoofer (in an apartment). My center (RC-3) is set at 80Hz I believe.
I would probably run the RF-82's or RF-7's full range, but others might disagree as they are not truly full range (20Hz-20kHz). The frequency response of the center you have is 59Hz-24KHz ± 3dB, so I would cross it a little above that. The Polk monitor 60's should probably stay at 80Hz, although its hard to tell because Polk's specifications don't make a ton of sense.
A new sub and new towers would make a killer system