I hate to say this, but none of those will work particularly well. First of all concrete is commonly thought of as the ultimate isolator of sound but lab tests show this is far from true, especially with block walls.
#1 Any constrained layer damping material needs to be placed between two layers of mass with similar flexibility. Concrete and drywall are not similar, obviously.
#2 adding 1" of airspace might be better, but a small air cavity will cause problems. The system is still rigid and coupled, and will definately makes things worse at some frequencies. That new drywall layer + airspace will create an amplifier for certain frequencies, typically higher freqs.
#3 Adding GG will help, but only a small amount. Still have the small air cavity, and rigid, coupled framing.
This has been tested and documented by the National Research Council of Canada. Really the only thing you can do that is effective would be to install a new framed wall that does not contact the concrete wall. Minimum 2x3 steel stud, at least 1/2" away from concrete. Now you have introduced decoupling.
Add R11 or R13 fiberglass. Now you have introduced absorption.
Add double 5/8" drywall. Standard stuff, nothing exotic. Now you have introduced (more) mass.
Add the GG at this point. Now you have introduced damping.
That's not the answer you wanted, but that's why many people choose to do nothing.