Prioritize your restoration project. Start with the most critical aspects.
Cap replacement should be high on your list. You could replace the entire networks, but it's the old caps that are out of spec that cause issues. Some of the old Klipsch farts prefer PIO to keep the vintage sound, while other prefer the lower esr (not to mention cost) of polys, which are a bit less forgiving. Don't fall for any audiophoolishness with the cap choice, this should not be an expensive mod. It's more maintenance than modification.
While you're in there, check the cab's integrity. You could put some dynamat on the horns if you like, not sure it will do much, but maybe.
I don't recommend more extensive mods (different drivers, completely different types of networks) as they become more of an unnecessary re-engineering project IMO, and will reduce the speakers' resale value. Heresy speakers in good cosmetic condition will fetch several hundred dollars.
Even in top form, they won't extend much above 17khz. Nor will they dig deep, dropping off ~60 hz (at least they're sealed, so the roll off does have useful output below that...they like corners). But they should be quite dynamic in between. They're fun. They're an easy load, can be driven with about anything.
HERE is a useful resource for your Klipsch aftermarket needs. (No affiliation. Bob's a straight shooter.)