The 603s are not really full range and only go down to 48Hz according to the specs. Not entirely sure if this is -3dB, -6dB or -10dB point, the datasheet is unclear, regardless you probably need a sub to round off the bottom end, especially for movies. A crossover of probably 60Hz or above should be used
The Polk goes down to 53Hz and so you should used at least 60Hz and probably 80Hz would work better.
I really won't comment on the Bose but they usually give wildly inaccurate range specs, if they give them at all. I would start with at least 80Hz and likely go above 100Hz.
With the setup as is, right now all the bass is going through the B&Ws. How well does it work in direct mode with stereo sources, ie music? Are they against the wall or out away a couple of feet?
A friend of mine has a pair these and we needed to bung the ports, oddly it was the rear port which is actually for the mid driver, he is in a small room, say 10x15. I found they image very easily and it is a small Yamaha AVR he is using to drive them, but only in stereo, with a slight toe in.